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Creators/Authors contains: "Chernowsky, Colleen_P"

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  1. ; ; (, Angewandte Chemie International Edition)
    Abstract Herein, we disclose that electrochemical stimulation induces new photocatalytic activity from a range of structurally diverse conventional photocatalysts. These studies uncover a new electron‐primed photoredox catalyst capable of promoting the reductive cleavage of strong C(sp2)−N and C(sp2)−O bonds. We illustrate several examples of the synthetic utility of these deeply reducing but otherwise safe and mild catalytic conditions. Finally, we employ electrochemical current measurements to perform a reaction progress kinetic analysis. This technique reveals that the improved activity of this new system is a consequence of an enhanced catalyst stability profile. 
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